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The effects of the substituents on the spectroscopic properties of 1-10 were examd. as a function of Tolman’s electronic parameter (╧Зi) for the substituents on silicon. The IR stretching frequency, ╬╜(Si-H), and the NMR coupling consts., 2JSiP and 1JSiH, exhibit a linear relationship with .sum.╧Зi, consistent with Bent’s rule. However, when the NMR resonances SiR3 ╬┤(29Si), SiH ╬┤(1H), and SiMe ╬┤(13C) were examd. as a function of .sum.╧Зi, the silyl groups differentiated into three classes: dichlorosilyl, monochlorosilyl, and “non-chlorosilyl”; within each class a linear but inverse relationship with .sum.╧Зi was obsd. 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